My personal favourites are the Bolland, Miller, Perez, and Arkham Asylum Batman pieces, and I love both the Jim Lee and Bermejo Jokers as well. You can still pick up the Jim Lee Joker pretty reasonably, but I think the Bermejo Joker is starting to command some high prices now, so if you see that for a decent price that may be one to grab as well...if you like Joker pieces.
And yeah, if you like it, grab the Mignola re-issue while you can, it's on the rise, just like the original.
But most of all, I'd just say collect the pieces and artists that you are a fan of, and just enjoy. Best of luck.
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